| Character | How to unlock
|
|---|
| A.I.M. Agent | Complete Level 10: That Sinking Feeling.
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| Abomination | Complete Level 4: Rock up at the Lock up.
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| Agent Coulson | Complete Bonus Level: Tabloid Tidy UP.
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| Aldrich Killian | Complete Level 5: Rebooted, Resuited.
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| Ant-Man | Collect his token in the Industrial District.
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| Archangel | Collect his token south of the X-Mansion, to the south of giant billboard.
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| Arnim Zola | Complete Level 6: Red Head Detention.
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| Beast | Complete Level 8: Juggernauts and Crosses.
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| Beetle | Collect his token a block east of the central park lake.
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| Black Cat | Collect her token below Lady Liberty on the map in a cat pet shop (requires Spider Man to unlock).
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| Black Widow | Complete Level 3: Exploratory Laboratory.
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| Blob | Complete Bonus Level: Put Up Your Dukes.
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| Captain America | Complete Level 2: Times Square Off.
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| Captain America (Comics) | Complete Bonus Level: The Brick Apple.
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| Captain Britain | Complete Bonus Level: The Brick Apple.
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| Colossus | Collect Colossus token in the front right courtyard of the X-Mansion.
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| Cyclops | Complete Level 8: Juggernauts and Crosses.
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| Damage Control | Put the out fires on the SHIELD Helicarrier deck with the water gun.
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| Deadpool | Collect all Deadpool Red Bricks.
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| Doc Ock | Complete Level 2: Times Square Off.
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| Doc Ock (Ultimate) | Complete Bonus Level: Tabloid Tidy UP.
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| Doombot | Complete Level 9: Doctor in the House.
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| Drax the Destroyer | Complete the story, then complete his 3 missions.
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| Electro | Complete Bonus Level: A Shock Withdrawal.
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| Frost Giant | Complete Level 7 - Bifrosty Reception.
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| Galactus (Minifig) | Complete Level 15: The Good, the Bad and the Hungry.
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| Gambit | Complete his 3 missions.
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| Gamora | Complete the story, then complete the first mission you get from Drax.
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| Green Goblin | Complete Level 9: Doctor in the House.
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| Groot | Complete the story, then complete his 3 missions.
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| H.E.R.B.I.E. | Complete Level 2: Times Square Off.
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| Hawkeye | Complete Level 3: Exploratory Laboratory.
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| Howard the Duck | Complete Bonus Level: Nuff Said.
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| Hulk | Complete Level 1: Sand Central Station.
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| Human Torch | Complete Level 6: Red Head Detention.
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| Iceman | Complete Level 8: Juggernauts and Crosses.
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| Invisible Woman | Complete Level 9: Doctor in the House.
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| Iron Fist | Complete race mission with Blade, then win the fight with ice dudes in the next Blade mission.
|
| Iron Man (Heroic Age) | Complete Bonus Level: New York Event.
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| Iron Man (Hulkbuster) | Land on "S" sign landing platform, then take out all the airvents that are all around the "S" sign.
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| Iron Man MK I | Complete Level 5: Rebooted, Resuited.
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| Iron Man MK VI | Complete Level 1: Sand Central Station.
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| Iron Man MK VII | Complete Bonus Level: House Party Protocol.
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| Iron Man MK XLVII | Complete Level 5: Rebooted, Resuited.
|
| Iron Man MK XVII | Complete Bonus Level: House Party Protocol.
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| Jean Grey | Complete Level 8: Juggernauts and Crosses.
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| Juggernaut | Complete Level 8: Juggernauts and Crosses.
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| Kraven the Hunter | Shoot the five targets next to the Godzilla-looking icon at the Central Park.
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| Loki | Complete Level 15: The Good, the Bad and the Hungry.
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| M.O.D.O.K. | Complete Level 10: That Sinking Feeling.
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| Magneto | Complete Level 13: Magnetic Personality.
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| Maria Hill | Complete her 3 missions on the Helicarrier.
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| Mister Fantastic | Complete Level 2: Times Square Off.
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| Mysterio | Complete Bonus Level: Thrill of the Chess.
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| Mystique | Complete Level 12: Rapturous Rise.
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| Nick Fury | Complete Level 9: Doctor in the House.
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| Nova | Complete foot race mission with him at the east of the giant Godzilla icon in the Central Park.
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| Professor Xavier | Complete his 3 missions behind the X-Mansion.
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| Psylocke | Complete all Captain Britain missions.
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| Pyro | Complete Level 8: Juggernauts and Crosses.
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| Red Skull | Complete Level 6: Red Head Detention.
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| Rhino | Complete Level 12: Rapturous Rise.
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| Rocket Raccoon | Complete his 3 missions.
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| Ronan the Accuser | Find hidden path behind the statue south of his icon.
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| Sandman | Complete Level 1: Sand Central Station.
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| Silver Surfer | Complete his 3 missions.
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| Spider-Man | Complete Level 1: Sand Central Station.
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| Spider-Woman | Collect her token west of the park on the southern most part of the island.
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| Squirrel Girl | Collect her token on the docks northwest of the Put Up Your Dukes bonus mission.
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| Stan Lee | Rescue all 50 Stan Lee in Peril.
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| Star-Lord | Complete his 3 missions.
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| Storm | Complete Level 8: Juggernauts and Crosses.
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| The Destroyer (Minifig) | Complete Level 7: Bifrosty Reception.
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| The Mandarin | Complete Level 5: Rebooted, Resuited.
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| Thing | Complete Level 9: Doctor in the House.
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| Thor | Complete Level 7: Bifrosty Reception.
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| Tony Stark | Complete Level 5: Rebooted, Resuited.
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| Tony Stark (Underwear) | Complete Level 4: Rock up at the Lock up.
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| Union Jack | Complete Bonus Level: The Brick Apple.
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| Venom | Complete Level 3: Exploratory Laboratory.
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| Wasp | Collect his token one block south of the Oscorp Building.
|
| Wolverine | Complete Level 4: Rock up at the Lock up.
|
